Prepare an empty datatatable with build datatable and configure 2 cols, Country, Count - dtResult
Assign Activity:
dtResult =
(From d in YourDataTableVar.AsEnumerable
Group d by k=d(0).ToString.ToUpper.Trim into grp=Group
Let ra = new Object(){k, grp.Count}
Select r = dtResult.Rows.Add(ra)).CopyToDataTAble