@arun.v7
keep one thing in mind:
grouping on first column and sorting on first column will create the series
111,222 …
sorting on second column you should decide the criteria for the sorting Ascending, Descending
maybe the following is needed:
(From d in dtAdultTable.AsEnumerable
Let s1 = CInt(d("GN").toString.Trim)
Let s2 = d("JMBWN").toString.Trim
Order by s1,s2 DESCENDING
Select r=d).CopyToDataTable
But we cannot do:

UPD1 - Visualizations:
